To play Ascension via emulation, you must use the on a high-end PC. For the PPSSPP emulator, you should instead look for the two legitimate PSP titles: Chains of Olympus and Ghost of Sparta God of War: Ascension (Original PS3 Review)
If you find a website claiming to offer a "God of War Ascension PPSSPP ISO," it is likely one of two things: God Of War Ascension Ppsspp Iso File Download --INSTALL
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A "re-skinned" version of God of War: Chains of Olympus or Ghost of Sparta made to look like Ascension. Malware: A fake file intended to harm your device. What God of War Games CAN You Play on PPSSPP? To play Ascension via emulation, you must use
God of War: Ascension is an action-adventure game developed by Sony Santa Monica Studio and published by Sony Computer Entertainment. The game was initially released for the PlayStation 3 in 2013. However, with the help of PPSSPP, a popular PSP emulator for Android and PC, you can now experience this thrilling game on your device. What God of War Games CAN You Play on PPSSPP
I notice you're looking for a download related to God of War: Ascension for PPSSPP. I should clarify a few important points:
How to Play God of War Ascension on PC - RPCS3 Full Tutorial